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Haglund, Richard F.
Member, VINSE Advisory Committee

Member, VINSE Facility User Committee
Stevenson Professor of Physics
Director, VINSE Nano Optics Facility

Research Information

Nonlinear laser interactions with nanostructured materials; ultrafast laser spectroscopy of metal and semiconductor nanocrystals; plasmonics in metal and metal-oxide nanostructures; fabrication of metal and oxide nanocrystal films and nanostructured arrays; ultrafast infrared laser deposition of thin films; free-electron laser applications in materials science; infrared pulsed laser deposition of polymers. Principal investigator, DOE Nanoscience, Engineering and Technology (NSET) project; co-principal investigator in NSF-GOALI project (Vanderbilt, Oak Ridge National Laboratory, Alcoa Technology Laboratories); co-Principal Investigator, W. M. Keck Foundation Free-Electron Laser Center at Vanderbilt University.


Selected Publications

Detecting Nanoscale Size Dependence in VO2 Phase Transition Using a Split-Ring Resonator Metamaterial. Appavoo, K; Haglund, RF, NANO LETTERS, 11, 1025-1031 , (2011)

Mechanisms of Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation. Torres, RD; Johnson, SL; Haglund, RF; Hwang, J; Burn, PL; Holloway, PH, CRITICAL REVIEWS IN SOLID STATE AND MATERIALS SCIENCES, 36, 16-45 , (2011)

Ultrafast compact silicon-based ring resonator modulators using metal-insulator switching of vanadium dioxide

. Nag, J; Ryckman, JD; Hertkorn, MT; Choi, BK; Haglund, RF; Weiss, SM, PROCEEDINGS - SPIE, 7597, 759710 , (2010)

Coupling of photoluminescent centers in ZnO to localized and propagating surface plasmons. Haglund, RF; Lawrie, BJ; Mu, R, THIN SOLID FILMS, 518, 4637-4643 , (2010)

Nonreciprocal switching of VO2 thin films on microstructured surfaces. Karakurt, I; Adams, CH; Leiderer, P; Boneberg, J; Haglund, RF, OPTICS LETTERS, 35, 1506-1508 , (2010)

Plasmonic Response of Nanoscale Spirals. Ziegler, JI; Haglund, RF, NANO LETTERS, 10, 3013-3018 , (2010)

Single-particle plasmon resonance spectroscopy of phase transition in vanadium dioxide. Lei, DY; Appavoo, K; Sonnefraud, Y; Haglund, RF; Maier, SA, OPTICS LETTERS, 35, 3988-3990 , (2010)

Thermal Confinement and Temperature-Dependent Absorption in Resonant Infrared Ablation of Frozen Liquid Targets. Bubb, DM; Johnson, SL; Collins, B; Haglund, RF, JOURNAL OF PHYSICAL CHEMISTRY C, 114, 5611-5616 , (2010)

Confocal Raman Microscopy across the Metal-Insulator Transition of Single Vanadium Dioxide Nanoparticles. Donev, EU; Lopez, R; Feldman, LC; Haglund, RF, NANO LETTERS, 9, 702-706 , (2009)

Dichroism in Ag nanoparticle composites with bimodal size distribution. Magruder, RH; Robinson, SJ; Smith, C; Meldrum, A; Halabica, A; Haglund, RF, JOURNAL OF APPLIED PHYSICS, 105, 024303 , (2009)

Effects of the absorption coefficient on resonant infrared laser ablation of poly(ethylene glycol). Johnson, SL; Schriver, KE; Haglund, RF; Bubb, DM, JOURNAL OF APPLIED PHYSICS, 105, 024901 , (2009)

Enhancement of ZnO photoluminescence by localized and propagating surface plasmons. Lawrie, BJ; Haglund, RF; Mu, R, OPTICS EXPRESS, 17, 2565-2572 , (2009)

Excitation and detection of surface acoustic phonon modes in Au/Al2O3 multilayers. Halabica, A; Pantelides, ST; Haglund, RF; Magruder, RH; Meldrum, A, PHYSICAL REVIEW B, 80, 165422 , (2009)

Phase explosion and recoil-induced ejection in resonant-infrared laser ablation of polystyrene. Johnson, SL; Bubb, DM; Haglund, RF, APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 96, 627-635 , (2009)

Size effects in the structural phase transition of VO2 nanoparticles studied by surface-enhanced Raman scattering. Donev, EU; Ziegler, JI; Haglund, RF; Feldman, LC, JOURNAL OF OPTICS A-PURE AND APPLIED OPTICS, 11, 125002 , (2009)

Universal optical response of Si-Si bonds and its evolution from nanoparticles to bulk crystals. Idrobo, JC; Halabica, A; Magruder, RH; Haglund, RF; Pennycook, SJ; Pantelides, ST, PHYSICAL REVIEW B, 79, 125322 , (2009)

Modulation of the gold particle-plasmon resonance by the metal-semiconductor transition of vanadium dioxide. Suh, JY; Donev, EU; Ferrara, DW; Tetz, KA; Feldman, LC; Haglund, RF, JOURNAL OF OPTICS A-PURE AND APPLIED OPTICS, 10, 055202 , (2008)

Pulsed infrared laser annealing of gold nanoparticles embedded in a silica matrix. Halabica, A; Idrobo, JC; Pantelides, ST; Magruder, RH; Pennycook, SJ; Haglund, RF, JOURNAL OF APPLIED PHYSICS, 103, 083545 , (2008)

Synthesis of vanadium dioxide thin films and nanoparticles. Nag, J; Haglund, RF, JOURNAL OF PHYSICS-CONDENSED MATTER, 20, 264016 , (2008)

Coherent structural dynamics and electronic correlations during an ultrafast insulator-to-metal phase transition in VO2. Kubler, C; Ehrke, H; Huber, R; Lopez, R; Halabica, A; Haglund, RF; Leitenstorfer, A, PHYSICAL REVIEW LETTERS, 99, 116401 , (2007)

Deposition of polyimide precursor by resonant infrared laser ablation. Dygert, NL; Gies, AP; Schriver, KE; Haglund, RF, APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 89, 481-487 , (2007)

Electronic and Optical Properties of Polymer Thin Films Deposited by Resonant Infrared Laser Ablation. Haglund, RF; Johnsonand, SL; Park, HK, JOURNAL OF LASER MICRO NANOENGINEERING, 2, 234-240 , (2007)

Properties of conductive polymer films deposited by infrared laser ablation. Johnson, SL; Park, HK; Haglund, RF, APPLIED SURFACE SCIENCE, 253, 6430-6434 , (2007)

Second harmonic generation from resonantly excited arrays of gold nanoparticles. McMahon, MD; Ferrara, D; Bowie, CT; Lopez, R; Haglund, RF, APPLIED PHYSICS B-LASERS AND OPTICS, 87, 259-265 , (2007)

Transmission increase upon switching of VO2 thin films on microstructured surfaces. Karakurt, I; Boneberg, J; Leiderer, P; Lopez, R; Halabica, A; Haglund, RF, APPLIED PHYSICS LETTERS, 91, 091907 , (2007)

X-ray diffraction studies of the growth of vanadium dioxide nanoparticles. Pauli, SA; Herger, R; Willmott, PR; Donev, EU; Suh, JY; Haglund, RF, JOURNAL OF APPLIED PHYSICS, 102, 073527 , (2007)

Mode-specific effects in resonant infrared ablation and deposition of polystyrene. Bubb, DM; Johnson, SL; Belmont, R; Schriver, KE; Haglund, RF; Antonacci, C; Yeung, LS, APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 83, 147-151 , (2006)

Modulated optical transmission of subwavelength hole arrays in metal-VO2 films. Suh, JY; Donev, EU; Lopez, R; Feldman, LC; Haglund, RF, APPLIED PHYSICS LETTERS, 88, 133115 , (2006)

Optical properties of subwavelength hole arrays in vanadium dioxide thin films. Donev, EU; Suh, JY; Villegas, F; Lopez, R; Haglund, RF; Feldman, LC, PHYSICAL REVIEW B, 73, 201401 , (2006)

Second-harmonic generation from arrays of symmetric gold nanoparticles. McMahon, MD; Lopez, R; Haglund, RF; Ray, EA; Bunton, PH, PHYSICAL REVIEW B, 73, 041401 , (2006)

Two-dimensional current percolation in nanocrystalline vanadium dioxide films. Rozen, J; Lopez, R; Haglund, RF; Feldman, LC, APPLIED PHYSICS LETTERS, 88, 081902 , (2006)

Applications of free-electron lasers in the biological and material sciences. Edwards, GS; Allen, SJ; Haglund, RF; Nemanich, RJ; Redlich, B; Simon, JD; Yang, WC, PHOTOCHEMISTRY AND PHOTOBIOLOGY, 81, 711-735 , (2005)

Photoinduced phase transition in VO2 nanocrystals: ultrafast control of surface-plasmon resonance. Rini, M; Cavalleri, A; Schoenlein, RW; Lopez, R; Feldman, LC; Haglund, RF; Boatner, LA; Haynes, TE, OPTICS LETTERS, 30, 558-560 , (2005)

Rapid tarnishing of silver nanoparticles in ambient laboratory air. Mcmahon, M; Lopez, R; Meyer, HM; Feldman, LC; Haglund, RF, APPLIED PHYSICS B-LASERS AND OPTICS, 80, 915-921 , (2005)

Dislocation arrangements in pentacene thin films. Nickel, B; Barabash, R; Ruiz, R; Koch, N; Kahn, A; Feldman, LC; Haglund, RF; Scoles, G, PHYSICAL REVIEW B, 70, 125401 , (2004)

Infrared near-field microscopy with the Vanderbilt free electron laser: overview and perspectives. Vobornik, D; Margaritondo, G; Sanghera, JS; Thielen, P; Aggarwal, ID; Ivanov, B; Miller, JK; Haglund, R; Tolk, NH; Congiu-Castellano, A; Rizzo, MA; Piston, DW; Somma, F; Baldacchini, G; Bonfigli, F; Marolo, T; Flora, F; Montereali, RM; Faenov, A; Pikuz, T; Longo, G; Mussi, V; Generosi, R; Luce, M; Perfetti, P; Cricenti, A, INFRARED PHYSICS & TECHNOLOGY, 45, 409-416 , (2004)

Optical nanospectroscopy applications in material science. Cricenti, A; Longo, G; Ustione, A; Mussi, V; Generosi, R; Luce, M; Rinaldi, M; Perfetti, P; Vobornik, D; Margaritondo, G; Sanghera, JS; Thielen, P; Aggarwal, ID; Ivanov, B; Miller, JK; Haglund, R; Tolk, NH; Congiu-Castellano, A; Rizzo, MA; Piston, DW; Somma, F; Baldacchini, G; Bonfigli, F; Marolo, T; Flora, F; Montereali, RM; Faenov, A; Pikuz, T, APPLIED SURFACE SCIENCE, 234, 374-386 , (2004)

Optical nonlinearities in VO2 nanoparticles and thin films. Lopez, R; Haglund, RF; Feldman, LC; Boatner, LA; Haynes, TE, APPLIED PHYSICS LETTERS, 85, 5191-5193 , (2004)

Picosecond pulsed laser deposition at high vibrational excitation density: the case of poly(tetrafluoroethylene). Papantonakis, MR; Haglund, RF, APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 79, 1687-1694 , (2004)

Semiconductor to metal phase transition in the nucleation and growth of VO2 nanoparticles and thin films. Suh, JY; Lopez, R; Feldman, LC; Haglund, RF, JOURNAL OF APPLIED PHYSICS, 96, 1209-1213 , (2004)

Size-dependent optical properties of VO2 nanoparticle arrays. Lopez, R; Feldman, LC; Haglund, RF, PHYSICAL REVIEW LETTERS, 93, 177403 , (2004)

Switchable reflectivity on silicon from a composite VO2-SiO2 protecting layer. Lopez, R; Boatner, LA; Haynes, TE; Haglund, RF; Feldman, LC, APPLIED PHYSICS LETTERS, 85, 1410-1412 , (2004)

Dynamic scaling, island size distribution, and morphology in the aggregation regime of submonolayer pentacene films. Ruiz, R; Nickel, B; Koch, N; Feldman, LC; Haglund, RF; Kahn, A; Family, F; Scoles, G, PHYSICAL REVIEW LETTERS, 91, 136102 , (2003)

Free-electron-laser-based biophysical and biomedical instrumentation. Edwards, GS; Austin, RH; Carroll, FE; Copeland, ML; Couprie, ME; Gabella, WE; Haglund, RF; Hooper, BA; Hutson, MS; Jansen, ED; Joos, KM; Kiehart, DP; Lindau, I; Miao, J; Pratisto, HS; Shen, JH; Tokutake, Y; van der Meer, AFG; Xie, A, REVIEW OF SCIENTIFIC INSTRUMENTS, 74, 3207-3245 , (2003)

Mid-infrared laser ablation of a hard biocomposite material: mechanistic studies of pulse duration and interface effects. Ivanov, B; Hakimian, AM; Peavy, GM; Haglund, RF, APPLIED SURFACE SCIENCE, 208, 77-84 , (2003)

Particle-solid interactions and 21st century materials science. Feldman, LC; Lupke, G; Tolk, NH; Lopez, R; Haglund, RF; Haynes, TE; Boatner, LA, NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 212, 1-7 , (2003)

Pentacene ultrathin film formation on reduced and oxidized Si surfaces. Ruiz, R; Nickel, B; Koch, N; Feldman, LC; Haglund, RF; Kahn, A; Scoles, G, PHYSICAL REVIEW B, 67, 125406 , (2003)

Effect of ablation parameters on infrared pulsed laser deposition of poly(ethylene glycol) films. Bubb, DM; Papantonakis, MR; Toftmann, B; Horwitz, JS; McGill, RA; Chrisey, DB; Haglund, RF, JOURNAL OF APPLIED PHYSICS, 91, 9809-9814 , (2002)

Four-wave-mixing phenomena associated with 700-fs-pumped potassium vapor. Garrett, WR; Haglund, RF; Ermer, DR; Deng, L; Payne, MG, LASER PHYSICS, 12, 1155-1160 , (2002)

Infrared laser ablation and ionization of water clusters and biomolecules from ice. Baltz-Knorr, ML; Schriver, KE; Haglund, RF, APPLIED SURFACE SCIENCE, 197, 11-16 , (2002)

Infrared laser desorption and ionization of polypeptides from a polyacrylamide gel. Baltz-Knorr, M; Ermer, DR; Schriver, KE; Haglund, RF, JOURNAL OF MASS SPECTROMETRY, 37, 254-258 , (2002)

Mechanisms of oxygen incorporation in indium-tin-oxide films deposited by laser ablation at room temperature. Morales-Paliza, MA; Haglund, RF; Feldman, LC, APPLIED PHYSICS LETTERS, 80, 3757-3759 , (2002)

Picosecond infrared laser desorption of biomolecules from ice.. Schriver, KE; Baltz-Knorr, ML; Haglund, RF, ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 224, U324-U324 , (2002)

Picosecond infrared matrix-assisted laser desorption/ionization mass spectrometry of organic molecules on sodium nitrate crystallites. Papantonakis, MR; Ermer, DR; Haglund, RF, APPLIED SURFACE SCIENCE, 197, 213-216 , (2002)

Pulsed laser deposition of conductive metallo-dielectric optical filters. Lopez, R; Ruiz, R; Haglund, RF; Feldman, LC, APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 74, 307-310 , (2002)

Resonant infrared pulsed laser deposition of thin biodegradable polymer films. Bubb, DM; Toftmann, B; Haglund, RF; Horwitz, JS; Papantonakis, MR; McGill, RA; Wu, PW; Chrisey, DB, APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 74, 123-125 , (2002)

Size effects in the structural phase transition of VO2 nanoparticles. Lopez, R; Haynes, TE; Boatner, LA; Feldman, LC; Haglund, RF, PHYSICAL REVIEW B, 65, 224113 , (2002)

Synthesis and characterization of size-controlled vanadium dioxide nanocrystals in a fused silica matrix. Lopez, R; Boatner, LA; Haynes, TE; Feldman, LC; Haglund, RF, JOURNAL OF APPLIED PHYSICS, 92, 4031-4036 , (2002)

Temperature-controlled surface plasmon resonance in VO2 nanorods. Lopez, R; Haynes, TE; Boatner, LA; Feldman, LC; Haglund, RF, OPTICS LETTERS, 27, 1327-1329 , (2002)

Vapor deposition of polystyrene thin films by intense laser vibrational excitation. Bubb, DM; Papantonakis, MR; Horwitz, JS; Haglund, RF; Toftmann, B; McGill, RA; Chrisey, DB, CHEMICAL PHYSICS LETTERS, 352, 135-139 , (2002)

What do matrix-assisted laser desorption/ionization mass spectra reveal about ionization mechanisms?. Papantonakis, MR; Kim, J; Hess, WP; Haglund, RF, JOURNAL OF MASS SPECTROMETRY, 37, 639-647 , (2002)

Enhanced hysteresis in the semiconductor-to-metal phase transition of VO2 precipitates formed in SiO2 by ion implantation. Lopez, R; Boatner, LA; Haynes, TE; Haglund, RF; Feldman, LC, APPLIED PHYSICS LETTERS, 79, 3161-3163 , (2001)

Intensity dependence of cation kinetic energies from 2,5-dihydroxybenzoic acid near the infrared matrix-assisted laser desorption/ionization threshold. Ermer, DR; Baltz-Knorr, M; Haglund, RF, JOURNAL OF MASS SPECTROMETRY, 36, 538-545 , (2001)

Molecular identification of mixed tank-waste compounds by mass spectrometry.. Papantonakis, MR; Haglund, RF; Hess, WP; Ermer, DR, ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 222, U34-U34 , (2001)

Nanocomposite materials formed by ion implantation. Meldrum, A; Haglund, RF; Boatner, LA; White, CW, ADVANCED MATERIALS, 13, 1431-+ , (2001)

Resonant infrared pulsed-laser deposition of a sorbent chemoselective polymer. Bubb, DM; Horwitz, JS; McGill, RA; Chrisey, DB; Papantonakis, MR; Haglund, RF; Toftmann, B, APPLIED PHYSICS LETTERS, 79, 2847-2849 , (2001)

Resonant infrared pulsed-laser deposition of polymer films using a free-electron laser. Bubb, DM; Horwitz, JS; Callahan, JH; McGill, RA; Houser, EJ; Chrisey, DB; Papantonakis, MR; Haglund, RF; Galicia, MC; Vertes, A, JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-AN INTERNATIONAL JOURNAL DEVOTED TO VACUUM SURFACES AND FILMS, 19, 2698-2702 , (2001)


Phone: 615-322-7964
Email: richard.haglund@vanderbilt.edu
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